%0 Journal Article %K Electrons %K Magnetism %K Free electron lasers %K X-ray Diffraction %K Magnetic moments %K Spin-orbit couplings %K Optical pumping %K Time measurement %K Iridates %K Localized magnetic moments %K Relaxation time scale %K Resonant diffraction %K Resonant x-ray diffraction %K Time resolved studies %K X-ray studies %A O Krupin %A G.L Dakovski %A B.J Kim %A J.W Kim %A J Kim %A S Mishra %A Y.-D Chuang %A C.R Serrao %A W.-S Lee %A W.F Schlotter %A M.P Minitti %A D Zhu %A D Fritz %A M Chollet %A Ramamoorthy Ramesh %A S.L Molodtsov %A J.J Turner %B Journal of Physics Condensed Matter %D 2016 %G eng %I Institute of Physics Publishing %R 10.1088/0953-8984/28/32/32LT01 %T Ultrafast dynamics of localized magnetic moments in the unconventional Mott insulator Sr2IrO4 %V 28 %X We report a time-resolved study of the ultrafast dynamics of the magnetic moments formed by the states in Sr2IrO4 by directly probing the localized iridium 5d magnetic state through resonant x-ray diffraction. Using optical pump-hard x-ray probe measurements, two relaxation time scales were determined: a fast fluence-independent relaxation is found to take place on a time scale of 1.5 ps, followed by a slower relaxation on a time scale of 500 ps-1.5 ns. © 2016 IOP Publishing Ltd.