%0 Journal Article %K Model %K Target %K Measurements %K Measurement %K USA %K Surface %K Emission %K Pulse %K Velocity %K Experimental %K Algorithm %K Interferometry %K Material %K Ablation %K Laser %K Laser ablation %K Laser ablation %K Breakdown %K Time-resolved %K Time %K Ca %K E %K Form %K Plasma %K Solids %K Number %K Pulses %K Vapor %K C %K Metals %K Ionization %K Electron number densities %K Plasmas %K Picosecond %K Picosecond laser %K Picosecond laser ablation %K Density %K Pulsed laser %K Pulsed laser %K Targets %K Electron %K Electron number density %K Number density %K Order %K Ha %K Metal %K Dynamics %K Results %K Expansion %K Plume %K Atmosphere %K Physics %K Air %K Air breakdown %K Electron emission %K Electron-emission %K Forms %K Heat transfer %K Laser plasma %K Laser plasmas %K Pulsed laser ablation (PLA) %K Pulsed laser ablation (PLA) %K Theoretical-model %K Vapor plume %A Samuel S Mao %A Xianglei Mao %A Ralph Greif %A Richard E Russo %B Applied Physics Letters %D 2000 %F Laser %G eng %N 16 %P 2464-2466 %R 10.1063/1.1318239 %T Initiation of an early-stage plasma during picosecond laser ablation of solids %V 77 %2 LBNL-46390 %8 10/2000 %X

Picosecond time-resolved images of plasma initiation were recorded during pulsed-laser ablation of metal targets in an air atmosphere. An early-stage plasma was observed to form before the release of a material vapor plume. Close to the target surface, interferometry measurements indicate that the early-stage plasma has an electron number density on the order of 1020 cm-3. The longitudinal expansion of the ionization front for this plasma has a velocity 109 cm/s, during the laser pulse. In contrast, a material-vapor plume forms approximately 200 ps after the laser pulse, and it moves away from the target at 106 cm/s. The experimental observations of the early-stage plasma were simulated by using a theoretical model based on a two-fluids description of laser plasmas. The results indicate that the initiation of the plasma is due to air breakdown assisted by electron emission from the target.