TY - JOUR KW - Film KW - Temperature measurement KW - Manganese KW - Impedance KW - Article KW - Dielectric constant KW - Calcium ion KW - Lanthanide KW - Oxygen derivative KW - Chemical binding KW - Equilibrium constant AU - L.V Saraf AU - S.B Ogale AU - Z Chen AU - R.P Godfrey AU - T Venkatesan AU - Ramamoorthy Ramesh AB - Frequency-dependent capacitance measurements and transport measurements tuned to reveal system impedance have been performed on epitaxial thin films of Pr0.67Ca0.33MnO3. These reflect strong dielectric response features correlated to the various ordering transition temperatures in the system, namely, ∼220 K (charge ordering), ∼130 K (antiferromagnetic ordering), and ∼117 K (spin canting). An equally strong feature is also seen at ∼125 K, which does not correspond to any reported transition. The enhanced dielectric response at the transitions is attributed to the nonequilibrium transport and slow carrier reorganization dynamics defined by polaronic hopping and magnetic frustration. BT - Physical Review B - Condensed Matter and Materials Physics DO - 10.1103/PhysRevB.62.R11961 LA - eng M1 - 18 N1 - cited By 8 N2 - Frequency-dependent capacitance measurements and transport measurements tuned to reveal system impedance have been performed on epitaxial thin films of Pr0.67Ca0.33MnO3. These reflect strong dielectric response features correlated to the various ordering transition temperatures in the system, namely, ∼220 K (charge ordering), ∼130 K (antiferromagnetic ordering), and ∼117 K (spin canting). An equally strong feature is also seen at ∼125 K, which does not correspond to any reported transition. The enhanced dielectric response at the transitions is attributed to the nonequilibrium transport and slow carrier reorganization dynamics defined by polaronic hopping and magnetic frustration. PY - 2000 SP - R11961 EP - R11964 T2 - Physical Review B - Condensed Matter and Materials Physics TI - Correlation of large dielectric response with the ordering transitions in PR0.67Ca0.33MnO3 VL - 62 SN - 01631829 ER -