TY - JOUR KW - Electricity KW - Energy KW - Temperature KW - Pulsed laser deposition KW - Film KW - Laser KW - Magnetic field KW - Iron KW - Arrays KW - Nanostructured materials KW - Oxygen KW - Ferroelectric materials KW - Nanotechnology KW - Electric field KW - Article KW - Priority journal KW - Titanium KW - Magnetization KW - Magnets KW - Cobalt KW - Thermodynamics KW - Nanoparticle KW - Transducer KW - Magnet KW - Parameter KW - Barium compounds KW - Couplings KW - Magnetic order KW - Barium KW - Molecular interaction AU - H Zheng AU - J Wang AU - S.E Lofland AU - Z Ma AU - L Mohaddes-Ardabili AU - T Zhao AU - L Salamanca-Riba AU - S.R Shinde AU - S.B Ogale AU - F Bai AU - D Viehland AU - Y Jia AU - D.G Schlom AU - M Wuttig AU - A Roytburd AU - Ramamoorthy Ramesh AB - We report on the coupling between ferroelectric and magnetic order parameters in a nanostructured BaTiO3-CoFe2O4 ferroelectromagnet. This facilitates the interconversion of energies stored in electric and magnetic fields and plays an important role in many devices, including transducers, field sensors, etc. Such nanostructures were deposited on single-crystal SrTiO3 (001) substrates by pulsed laser deposition from a single Ba-Ti-Co-Fe-oxide target. The films are epitaxial in-plane as well as out-of-plane with self-assembled hexagonal arrays of CoFe 2O4 nanopillars embedded in a BaTiO3 matrix. The CoFe2O4 nanopillars have uniform size and average spacing of 20 to 30 nanometers. Temperature-dependent magnetic measurements illustrate the coupling between the two order parameters, which is manifested as a change in magnetization at the ferroelectric Curie temperature. Thermodynamic analyses show that the magnetoelectric coupling in such a nanostructure can be understood on the basis of the strong elastic interactions between the two phases. BT - Science DO - 10.1126/science.1094207 LA - eng M1 - 5658 N1 - cited By 1764 N2 - We report on the coupling between ferroelectric and magnetic order parameters in a nanostructured BaTiO3-CoFe2O4 ferroelectromagnet. This facilitates the interconversion of energies stored in electric and magnetic fields and plays an important role in many devices, including transducers, field sensors, etc. Such nanostructures were deposited on single-crystal SrTiO3 (001) substrates by pulsed laser deposition from a single Ba-Ti-Co-Fe-oxide target. The films are epitaxial in-plane as well as out-of-plane with self-assembled hexagonal arrays of CoFe 2O4 nanopillars embedded in a BaTiO3 matrix. The CoFe2O4 nanopillars have uniform size and average spacing of 20 to 30 nanometers. Temperature-dependent magnetic measurements illustrate the coupling between the two order parameters, which is manifested as a change in magnetization at the ferroelectric Curie temperature. Thermodynamic analyses show that the magnetoelectric coupling in such a nanostructure can be understood on the basis of the strong elastic interactions between the two phases. PY - 2004 SP - 661 EP - 663 T2 - Science TI - Multiferroic BaTiO3-CoFe2O4 Nanostructures VL - 303 SN - 00368075 ER -