TY - JOUR AU - M Huijben AU - L.W Martin AU - Y.-H Chu AU - M.B Holcomb AU - P Yu AU - G Rijnders AU - D.H.A Blank AU - Ramamoorthy Ramesh AB - Detailed analysis of transport, magnetism, and x-ray absorption spectroscopy measurements on ultrathin La0.7 Sr0.3 MnO3 films with thicknesses from 3 to 70 unit cells resulted in the identification of a lower critical thickness for a nonmetallic nonferromagnetic layer at the interface with the SrTiO3 (001) substrate of only three unit cells (∼12 Å). Furthermore, linear-dichroism measurements demonstrate the presence of a preferred (x2 - y2) in-plane orbital ordering for all layer thicknesses without any orbital reconstruction at the interface. A crucial requirement for the accurate study of these ultrathin films is a controlled growth process, offering the coexistence of layer-by-layer growth and bulklike magnetic/transport properties. © 2008 The American Physical Society. BT - Physical Review B - Condensed Matter and Materials Physics DO - 10.1103/PhysRevB.78.094413 LA - eng M1 - 9 N1 - cited By 289 N2 - Detailed analysis of transport, magnetism, and x-ray absorption spectroscopy measurements on ultrathin La0.7 Sr0.3 MnO3 films with thicknesses from 3 to 70 unit cells resulted in the identification of a lower critical thickness for a nonmetallic nonferromagnetic layer at the interface with the SrTiO3 (001) substrate of only three unit cells (∼12 Å). Furthermore, linear-dichroism measurements demonstrate the presence of a preferred (x2 - y2) in-plane orbital ordering for all layer thicknesses without any orbital reconstruction at the interface. A crucial requirement for the accurate study of these ultrathin films is a controlled growth process, offering the coexistence of layer-by-layer growth and bulklike magnetic/transport properties. © 2008 The American Physical Society. PY - 2008 T2 - Physical Review B - Condensed Matter and Materials Physics TI - Critical thickness and orbital ordering in ultrathin La0.7 Sr0.3 MnO3 films VL - 78 SN - 10980121 ER -