TY - JOUR KW - Methodology KW - Laser KW - Lasers KW - Aluminum KW - Electron KW - Electrodes KW - Chemistry KW - Electrons KW - Electrode KW - Nanoparticles KW - Near-field KW - Luminescence KW - Cerium KW - Nanostructures KW - Materials testing KW - Nanotechnology KW - Article KW - Surface properties KW - Surface property KW - Imaging techniques KW - Focused electron beams KW - Free standing membranes KW - Lithographic patterning KW - Mechanical scanning KW - Nano-optical KW - NanoPatterning KW - Near-field optical microscopy KW - Biological materials KW - Cathodoluminescence KW - Photoexcitation KW - Nanomaterial KW - Nanoparticle KW - Equipment design KW - Monte Carlo method KW - Optics KW - Optics and Photonics AU - D.M Kaz AU - C.G Bischak AU - C.L Hetherington AU - H.H Howard AU - X Marti AU - J.D Clarkson AU - C Adamo AU - D.G Schlom AU - Ramamoorthy Ramesh AU - S Aloni AU - D.F Ogletree AU - N.S Ginsberg AB - Demand for visualizing nanoscale dynamics in biological and advanced materials continues to drive the development of subdiffraction optical probes. While many strategies employ scanning tips for this purpose, we instead exploit a focused electron beam to create scannable nanoscale optical excitations in an epitaxially grown thin-film of cerium-doped yttrium aluminum perovskite, whose cathodoluminescence response is bright, robust, and spatially resolved to 18 nm. We also demonstrate lithographic patterning of the film's luminescence at the nanoscale. We anticipate that converting these films into free-standing membranes will yield a powerful near-field optical microscopy without the complication of mechanical scanning. © 2013 American Chemical Society. BT - ACS Nano DO - 10.1021/nn404911a LA - eng M1 - 11 N1 - cited By 12 N2 - Demand for visualizing nanoscale dynamics in biological and advanced materials continues to drive the development of subdiffraction optical probes. While many strategies employ scanning tips for this purpose, we instead exploit a focused electron beam to create scannable nanoscale optical excitations in an epitaxially grown thin-film of cerium-doped yttrium aluminum perovskite, whose cathodoluminescence response is bright, robust, and spatially resolved to 18 nm. We also demonstrate lithographic patterning of the film's luminescence at the nanoscale. We anticipate that converting these films into free-standing membranes will yield a powerful near-field optical microscopy without the complication of mechanical scanning. © 2013 American Chemical Society. PY - 2013 SP - 10397 EP - 10404 T2 - ACS Nano TI - Bright cathodoluminescent thin films for scanning nano-optical excitation and imaging VL - 7 SN - 19360851 ER -