TY - JOUR KW - Electric potential KW - Film KW - Spectroscopy KW - Resonance KW - Anisotropy KW - Iron KW - Scanning electron microscopy KW - Imaging KW - Hysteresis KW - Polarization KW - Electric field KW - Article KW - Magnetization KW - Bismuth KW - Cobalt KW - Electromagnetic field KW - Bismuth derivative KW - Electron spin resonance KW - Ferromagnetic resonance spectroscopy KW - Nanoanalysis KW - Strength KW - Surface property AU - Z Zhou AU - M Trassin AU - Yuan Gao AU - Yuan Gao AU - D Qiu AU - K Ashraf AU - T Nan AU - X Yang AU - S.R Bowden AU - D.T Pierce AU - M.D Stiles AU - J Unguris AU - M Liu AU - B.M Howe AU - G.J Brown AU - S Salahuddin AU - Ramamoorthy Ramesh AU - N.X Sun AB - Exchange coupled CoFe/BiFeO3 thin-film heterostructures show great promise for power-efficient electric field-induced 180° magnetization switching. However, the coupling mechanism and precise qualification of the exchange coupling in CoFe/BiFeO3 heterostructures have been elusive. Here we show direct evidence for electric field control of the magnetic state in exchange coupled CoFe/BiFeO3 through electric field-dependent ferromagnetic resonance spectroscopy and nanoscale spatially resolved magnetic imaging. Scanning electron microscopy with polarization analysis images reveal the coupling of the magnetization in the CoFe layer to the canted moment in the BiFeO3 layer. Electric field-dependent ferromagnetic resonance measurements quantify the exchange coupling strength and reveal that the CoFe magnetization is directly and reversibly modulated by the applied electric field through a ∼180° switching of the canted moment in BiFeO3. This constitutes an important step towards robust repeatable and non-volatile voltage-induced 180° magnetization switching in thin-film multiferroic heterostructures and tunable RF/microwave devices. © 2015 Macmillan Publishers Limited. All rights reserved. BT - Nature Communications DO - 10.1038/ncomms7082 LA - eng N1 - cited By 48 N2 - Exchange coupled CoFe/BiFeO3 thin-film heterostructures show great promise for power-efficient electric field-induced 180° magnetization switching. However, the coupling mechanism and precise qualification of the exchange coupling in CoFe/BiFeO3 heterostructures have been elusive. Here we show direct evidence for electric field control of the magnetic state in exchange coupled CoFe/BiFeO3 through electric field-dependent ferromagnetic resonance spectroscopy and nanoscale spatially resolved magnetic imaging. Scanning electron microscopy with polarization analysis images reveal the coupling of the magnetization in the CoFe layer to the canted moment in the BiFeO3 layer. Electric field-dependent ferromagnetic resonance measurements quantify the exchange coupling strength and reveal that the CoFe magnetization is directly and reversibly modulated by the applied electric field through a ∼180° switching of the canted moment in BiFeO3. This constitutes an important step towards robust repeatable and non-volatile voltage-induced 180° magnetization switching in thin-film multiferroic heterostructures and tunable RF/microwave devices. © 2015 Macmillan Publishers Limited. All rights reserved. PB - Nature Publishing Group PY - 2015 T2 - Nature Communications TI - Probing electric field control of magnetism using ferromagnetic resonance VL - 6 SN - 20411723 ER -