TY - JOUR KW - Electrons KW - Magnetism KW - Free electron lasers KW - X-ray Diffraction KW - Magnetic moments KW - Spin-orbit couplings KW - Optical pumping KW - Time measurement KW - Iridates KW - Localized magnetic moments KW - Relaxation time scale KW - Resonant diffraction KW - Resonant x-ray diffraction KW - Time resolved studies KW - X-ray studies AU - O Krupin AU - G.L Dakovski AU - B.J Kim AU - J.W Kim AU - James Hyungkwan Kim AU - S Mishra AU - Y.-D Chuang AU - C.R Serrao AU - W.-S Lee AU - W.F Schlotter AU - M.P Minitti AU - D Zhu AU - D Fritz AU - M Chollet AU - Ramamoorthy Ramesh AU - S.L Molodtsov AU - J.J Turner AB - We report a time-resolved study of the ultrafast dynamics of the magnetic moments formed by the states in Sr2IrO4 by directly probing the localized iridium 5d magnetic state through resonant x-ray diffraction. Using optical pump-hard x-ray probe measurements, two relaxation time scales were determined: a fast fluence-independent relaxation is found to take place on a time scale of 1.5 ps, followed by a slower relaxation on a time scale of 500 ps-1.5 ns. © 2016 IOP Publishing Ltd. BT - Journal of Physics Condensed Matter DO - 10.1088/0953-8984/28/32/32LT01 LA - eng M1 - 32 N1 - cited By 7 N2 - We report a time-resolved study of the ultrafast dynamics of the magnetic moments formed by the states in Sr2IrO4 by directly probing the localized iridium 5d magnetic state through resonant x-ray diffraction. Using optical pump-hard x-ray probe measurements, two relaxation time scales were determined: a fast fluence-independent relaxation is found to take place on a time scale of 1.5 ps, followed by a slower relaxation on a time scale of 500 ps-1.5 ns. © 2016 IOP Publishing Ltd. PB - Institute of Physics Publishing PY - 2016 T2 - Journal of Physics Condensed Matter TI - Ultrafast dynamics of localized magnetic moments in the unconventional Mott insulator Sr2IrO4 VL - 28 SN - 09538984 ER -