TY - JOUR KW - Modeling KW - Fuel cell KW - Water management KW - NSTF KW - Thin catalyst layer AU - Iryna V Zenyuk AU - Prodip K Das AU - Adam Z Weber AB - In this article, a two-dimensional, multiphase, transient model is introduced and used to explore the impact of catalyst-layer thickness on performance. In particular, the tradeoffs between water production and removal through transport or evaporation are highlighted, with a focus on low-temperature performance. For the latter, a case study of an ultra-thin catalyst layer is undergone to explore how various material properties alter the steady-state and startup performance of a cell. The findings provide understanding and guidance to optimize fuel-cell performance with thin electrodes. BT - Journal of The Electrochemical Society DA - 06/2016 DO - 10.1149/2.1161607jes IS - 7 LA - eng N2 - In this article, a two-dimensional, multiphase, transient model is introduced and used to explore the impact of catalyst-layer thickness on performance. In particular, the tradeoffs between water production and removal through transport or evaporation are highlighted, with a focus on low-temperature performance. For the latter, a case study of an ultra-thin catalyst layer is undergone to explore how various material properties alter the steady-state and startup performance of a cell. The findings provide understanding and guidance to optimize fuel-cell performance with thin electrodes. PY - 2016 SP - F691 EP - F703 ST - J. Electrochem. Soc. T2 - Journal of The Electrochemical Society TI - Understanding Impacts of Catalyst-Layer Thickness on Fuel-Cell Performance via Mathematical Modeling VL - 163 SN - 0013-4651 ER -