TY - JOUR
AU - Chengxiang Xiang
AU - Adam Z Weber
AU - Shane Ardo
AU - Alan Berger
AU - YiKai Chen
AU - Robert Coridan
AU - Katherine T Fountaine
AU - Sophia Haussener
AU - Shu Hu
AU - Riu Liu
AU - Nathan S Lewis
AU - Miguel A Modestino
AU - Matthew M Shaner
AU - Meenesh R Singh
AU - John C Stevens
AU - Ke Sun
AU - Karl Walczak
AB - <p>An integrated cell for the solar-driven splitting of water consists of multiple functional components and couples various photoelectrochemical (PEC) processes at different length and time scales. The overall solar-to-hydrogen (STH) conversion efficiency of such a system depends on the performance and materials properties of the individual components as well as on the component integration, overall device architecture, and system operating conditions. This Review focuses on the modeling- and simulation-guided development and implementation of solar-driven water-splitting prototypes from a holistic viewpoint that explores the various interplays between the components. The underlying physics and interactions at the cell level is are reviewed and discussed, followed by an overview of the use of the cell model to provide target properties of materials and guide the design of a range of traditional and unique device architectures.</p>
BT - Angewandte Chemie International Edition
DA - 10/2016
DO - 10.1002/anie.201510463
IS - 42
LA - eng
N2 - <p>An integrated cell for the solar-driven splitting of water consists of multiple functional components and couples various photoelectrochemical (PEC) processes at different length and time scales. The overall solar-to-hydrogen (STH) conversion efficiency of such a system depends on the performance and materials properties of the individual components as well as on the component integration, overall device architecture, and system operating conditions. This Review focuses on the modeling- and simulation-guided development and implementation of solar-driven water-splitting prototypes from a holistic viewpoint that explores the various interplays between the components. The underlying physics and interactions at the cell level is are reviewed and discussed, followed by an overview of the use of the cell model to provide target properties of materials and guide the design of a range of traditional and unique device architectures.</p>
PY - 2016
SP - 12974 
EP -  12988
ST - Angew. Chem. Int. Ed.
T2 - Angewandte Chemie International Edition
TI - Modeling, Simulation, and Implementation of Solar-Driven Water-Splitting Devices
VL - 55
ER -