TY - JOUR KW - Transport KW - Fuel cells KW - Catalyst layer KW - Infrared thermography KW - Manufacturing KW - Defect detection KW - Layer-thickness AU - Prodip K Das AU - Adam Z Weber AU - Guido Bender AU - Austin Manak AU - Daniel Bittinat AU - Andrew M Herring AU - Michael J Ulsh AB -

As fuel cells become more prominent, new manufacturing and production methods will need to be developed to deal efficiently and effectively with increased demand. One necessary component of this industrial growth is the accurate measurement of the variability in the manufacturing process. In this study, we present a diagnostic system that combines infrared thermography with a reactive-flow-through technique to detect catalyst-loading defects in fuel-cell gas-diffusion electrodes accurately with high spatial and temporal resolutions. Experimental results are compared with model predictions of thermal response with good agreement. Data analysis, operating-condition impacts, and detection limits are explored using both experiments and simulation. Overall, the results demonstrate the potential of this technique to measure defects on the millimeter length scale with temporal resolutions appropriate for use on a web-line. Thus we present the first development stage of a next-generation non-destructive diagnostic tool, which may be amenable to eventual use on roll-to-roll manufacturing lines.

BT - Journal of Power Sources DA - 09/2014 DO - 10.1016/j.jpowsour.2013.11.124 N2 -

As fuel cells become more prominent, new manufacturing and production methods will need to be developed to deal efficiently and effectively with increased demand. One necessary component of this industrial growth is the accurate measurement of the variability in the manufacturing process. In this study, we present a diagnostic system that combines infrared thermography with a reactive-flow-through technique to detect catalyst-loading defects in fuel-cell gas-diffusion electrodes accurately with high spatial and temporal resolutions. Experimental results are compared with model predictions of thermal response with good agreement. Data analysis, operating-condition impacts, and detection limits are explored using both experiments and simulation. Overall, the results demonstrate the potential of this technique to measure defects on the millimeter length scale with temporal resolutions appropriate for use on a web-line. Thus we present the first development stage of a next-generation non-destructive diagnostic tool, which may be amenable to eventual use on roll-to-roll manufacturing lines.

PY - 2014 SP - 401 EP - 411 ST - Journal of Power Sources T2 - Journal of Power Sources TI - Rapid detection of defects in fuel-cell electrodes using infrared reactive-flow-through technique UR - http://www.sciencedirect.com/science/article/pii/S0378775313019848 VL - 261 SN - 03787753 ER -