@article{34704, author = {Sarah A Berlinger and Samay Garg and Adam Z Weber}, title = {Multicomponent, multiphase interactions in fuel-cell inks}, abstract = {

Fuel-cell catalyst layers (CLs) are porous electrodes that are fabricated from CL inks: colloidal dispersions of catalyst particles and ion-conducting polymer (ionomer), dispersed in solvent(s). The complex interactions between the ink components ultimately dictate CL microstructure and electrochemical performance. To control the CL formation process and optimize fuel-cell performance, knowledge of these ink interactions is vital. In this review, we analyze data from ink-focused papers to elucidate how ink parameters (solvent type, ionomer-to-carbon ratio, etc.) impact ink interactions and CL performance. We then discuss these results in the context of the current understanding of two critical ink interactions: ionomer/solvent and ionomer/catalyst particle interactions.

}, year = {2021}, journal = {Current Opinion in Electrochemistry}, volume = {29}, pages = {100744}, month = {10/2021}, issn = {24519103}, doi = {10.1016/j.coelec.2021.100744}, language = {eng}, }