@article{33731, author = {V Nagarajan and C.S Ganpule and H Li and L Salamanca-Riba and A.L Roytburd and E.D Williams and Ramamoorthy Ramesh}, title = {Control of domain structure of epitaxial PbZr0.2Ti0.8O3 thin films grown on vicinal (001) SrTiO3 substrates}, abstract = {We have investigated the polydomain formation in 100-200-nm-thick PbZr0.2Ti0.8O3 epitaxial thin films on vicinally cut (100) oriented SrTiO3 substrates. Our results show that there is a preferential location of the nucleation of the a domains along the step edges of the underlying substrate. By piezo-response microscopy, we show that all a domains have their polarization aligned along the same direction. This result is in contrast to flat substrates where fourfold symmetry of a domains is observed. We observe that the critical thickness for a domain formation is much lower than that for PbZr0.2Ti0.8O3 films grown on flat substrates. We have developed a model based on minimization of elastic energy to describe the effect of localized stresses at step edges on the formation of a domains in the ferroelectric layer. © 2001 American Institute of Physics.}, year = {2001}, journal = {Applied Physics Letters}, volume = {79}, number = {17}, pages = {2805-2807}, issn = {00036951}, doi = {10.1063/1.1402645}, note = {cited By 25}, language = {eng}, }